re: Brad Pitt at the end of Seven: good or bad acting?

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I think it went along with his propensity towards reacting angrily and violently throughout the entire movie.

I mean shite, just look at his reaction about 10 seconds after opening Dante's Inferno.

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His aggression throughout the movie comes from his internal struggle with wrath.

Once he accepts his fate, whether he considers it successful or failure on his part, his personality should change. He should be calm and calculating in that moment.

ETA:
I should be a director